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Dielectric relaxation in chevron surface stabilized ferroelectric liquid crystals

机译:人字形表面稳定的铁电液体中的介电弛豫   晶体

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摘要

The dielectric response of surface stabilized ferroelectric liquid crystalswith chevron layer structure is studied within low and intermediate frequencyranges, characteristic for collective molecular excitations. By analyticallysolving the dynamic equation for collective molecular fluctuations under a weakalternating electric field, it is demonstrated that chevron cells stabilized byboth nonpolar and polar surface interactions undergo at medium frequencies twoDebye relaxation processes, connected with two chevron slabs, on opposite sidesof the interface plane. This result is confirmed, experimentally, making use ofthe electro-optic technique. Based on qualitative arguments supported bymicroscopic observations of zigzag defects at different frequencies andamplitudes of the external electric field, it is shown that, at lowfrequencies, the electro-optic response of chevron samples is determined bythree kinds of motions of zigzag walls. The first two dynamic categories arerelated to collective relaxation processes at weak fields, within smectic Alayers forming zigzag walls, and drift or creep motions of thick walls occuringat stronger field amplitudes. Dynamic processes of the third kind correspond tosliding of zigzag walls, which appear at yet stronger field amplitudes, butbelow the switching threshold.
机译:研究了在中低频范围内具有人字形结构的表面稳定铁电液晶结构人字形液晶的介电响应。通过解析弱交变电场下集体分子涨落的动力学方程,证明了通过非极性和极性表面相互作用稳定的人字形细胞在界面频率的相对侧经历了中频两次德拜弛豫过程,与两个人字形平板相连。实验结果是利用电光技术证实的。基于在不同频率和幅度的外部电场下对之字形缺陷进行显微观察的定性论证表明,在低频率下,人字形样品的电光响应是由三种之字形壁运动决定的。前两个动态类别与在形成锯齿形壁的近晶Alayer内的弱场处的集体弛豫过程有关,并且厚壁的漂移或蠕变运动在更强的场振幅下发生。第三类动态过程与之字形壁的滑动相对应,之字形出现在更强的场振幅处,但低于切换阈值。

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